厨余垃圾粉碎直排对反硝化过程氧化亚氮排放的影响研究OA
Study on effects of food waste crushing and direct discharge on nitrous oxide emissions during denitrification
厨余垃圾(FW)粉碎直排是一种可持续处理策略,但其对强温室气体氧化亚氮(N2O)排放的影响尚待评估.通过模拟FW粉碎直排入污水管网场景下的市政污水,探究了FW降解产物对反硝化过程中N2O排放的影响机制.实验结果表明,FW降解产物对硝酸盐与亚硝酸盐的还原速率均产生抑制作用,降幅分别为23.3%和19.0%,同时可使N2O还原速率提升9.8%.在非碳源限制条件下,FW降解产物增强了N2O还原酶(Nos)电子获取能力,加剧了反硝化酶系间的电子竞争,促使更多电子流向Nos.电子分布格局的改变是FW降解产物增强N2O还原能力的关键机制,有助于减少反硝化过程中N2O的积累.
Food waste(FW)crushing and direct discharge is a sustainable treatment strategy,but its impact on emissions of the potent greenhouse gas,nitrous oxide(N2O),remains to be assessed.The influence mecha-nism of FW degradation products on N2O emissions during denitrification were explored by simulating the mu-nicipal wastewater under the scenario of FW crushing and direct discharge into sewer.The experimental re-sults show that FW degradation products inhibit the reduction rates of both nitrate and nitrite,with the decline of 23.3%and 19.0%,respectively,while increasing the N2O reduction rate by 9.8%.Under the condition of non-limiting carbon source,FW degradation products enhance the electron acquisition capacity of N2O reduc-tase(Nos),and intensify the electron competition among denitrification reductases,prompting more electrons to flow towards Nos.The alteration of the electron distribution pattern is the key mechanism of the improve-ment of N2O reduction capability by FW degradation products,which helps to reduce N2O accumulation during denitrification.
刘轶文;李权;王晗炜;张树军;何衍英;王玉芬;朱婷婷
天津大学环境科学与工程学院,天津 300072天津大学环境科学与工程学院,天津 300072||北京城市排水集团有限责任公司科技研发中心,北京 100124天津大学环境科学与工程学院,天津 300072北京城市排水集团有限责任公司科技研发中心,北京 100124天津大学环境科学与工程学院,天津 300072天津大学环境科学与工程学院,天津 300072天津大学环境科学与工程学院,天津 300072
资源环境
氧化亚氮(N2O)生物脱氮厨余垃圾粉碎直排反硝化
nitrous oxide(N2O)biological nitrogen removalfood wastecrushing and direct dischargede-nitrification
《东南大学学报(自然科学版)》 2026 (8)
1176-1182,7
国家自然科学基金资助项目(52470108)国家重点研发计划资助项目(2024YFC3810200).
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