基于CO2关联的沈阳市NH3浓度影响因素探究OA
Influencing factors of NH3 concentration in Shenyang based on CO2 correlation
大气氨(NH3)对空气质量、生态系统和全球气候变化有直接和间接影响.NH3 并不是常规空气质量监测项目,这对沈阳市实施 NH3 管控带来较大的不确定性.文章以沈阳市为研究区域,通过随机森林、后向轨迹模型等方法,探究沈阳市夏冬两季 NH3 排放季节性变化规律、影响因素以及传输路径,并提出管控建议.结果表明:沈阳市夏季 NH3 浓度均值高于冬季.夏冬两季大气 NH3 浓度均呈现白天高、夜间低的规律,夏季 NH3 浓度变化波动较大,冬季 NH3 浓度变化则呈现单峰性.气象因素是影响沈阳市 NH3 浓度变化的主要因素,此外,CO2 和 CH4 浓度对 NH3 浓度的影响同样不可忽视.沈阳市夏冬两季NH3 浓度均同时受到周边多省份、国家的共同影响,夏季气团方向复杂,冬季则趋于单一.
Atmospheric ammonia(NH3)exerts direct and indirect impacts on air quality,ecosystems and global climate change.Since NH3 is not included in conventional air quality monitoring items,great uncertainties were brought to the implementation of ammonia pollution control in Shenyang.Taking Shenyang as the research area,this study explored the seasonal variation characteristics,influencing factors and transmission pathways of atmospheric NH3 in summer and winter,and put forward targeted control suggestions by adopting the random forest model,backward trajectory analysis and other methods.The results showed that the average NH3 concentration in Shenyang was higher in summer than in winter.In both seasons,atmospheric NH3 concentrations were characterized by higher values in the daytime and lower values at night.Large fluctuations in NH3 concentrations were observed in summer,while a single peak variation pattern was presented in winter.Meteorological factors were identified as the dominant factors affecting NH3 concentration variations.In addition,the influences of CO2 and CH4 concentrations on NH3 were also non-negligible.The atmospheric NH3 concentrations in Shenyang during summer and winter were jointly affected by surrounding provinces and neighboring countries.Air mass transport directions were complicated in summer,whereas a single transport direction was dominated in winter.
赵焕;王男;王姝欣;金东青;柳佳宏;李哲;刘闽;刘雨薇
辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136辽宁省沈阳生态环境监测中心,沈阳 110136||沈阳市碳监测技术研究重点实验室,沈阳 110136中国科学院金属研究所,沈阳 110136
资源环境
随机森林后向轨迹NH3CO2沈阳市
random forestbackward trajectoryNH3CO2Shenyang
《环境保护科学》 2026 (2)
129-135,7
辽宁省科学技术厅重点研发计划项目(2024JH2/102500098)
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