首页|期刊导航|人工晶体学报|快发光闪烁体上升沿精确测量及其在超快光电探测中的应用

快发光闪烁体上升沿精确测量及其在超快光电探测中的应用OA

Precise Measurement of Rising Edge in Fast Luminescent Scintillators and Its Application in Ultrafast Photodetection

中文摘要英文摘要

闪烁体作为将高能辐射转化为光信号的关键材料,其上升沿时间直接影响探测系统的时间分辨率,对于X射线自由电子激光(XFEL)设施中的脉冲诊断与束流监测,以及飞行时间正电子发射断层扫描(TOF-PET)等前沿领域至关重要.本工作旨在深入探讨闪烁体上升沿这一核心时间性能参数的重要性及其现有测量技术的瓶颈,并提出一种创新的高精度测量方案.研究利用355 nm皮秒脉冲激光,通过分光将光束分为触发光路与激发光路,并耦合光谱仪进行单色光选择,有效克服了激光脉冲抖动和弱荧光信号采集难题.实验测得,相比LYSO:Ce闪烁体的上升时间为(273.7±26.9)ps,新兴的CsPbCl3全无机钙钛矿闪烁体展现出低至(209.6±6.7)ps的超快上升时间,而衰减时间仅为(663.4±34.2)ps.这一百皮秒级的上升时间与超快响应特性,揭示了 CsPbCl3在吉赫兹高重频超快探测器领域的巨大潜力,为同步辐射和自由电子激光装置诊断提供了关键技术支撑,也为下一代超快闪烁体的筛选优化提供了关键方法与物理数据.

As a key material for converting high-energy radiation into optical signals,the rise time of scintillators directly affects the time resolution of detection systems.This parameter is crucial for cutting-edge applications such as pulse diagnostics and beam monitoring in X-ray free-electron laser(XFEL)facilities,as well as time-of-flight positron emission tomography(TOF-PET).This work thoroughly explores the significance of the rise time,a core temporal performance parameter of scintillators,highlights the limitations of existing measurement techniques,and proposes an innovative high-precision measurement scheme.The study utilizes a 355 nm picosecond pulsed laser,splitting the beam into trigger and excitation paths,coupled with a spectrometer for monochromatic light selection.This approach effectively overcomes challenges such as laser pulse jitter and weak fluorescence signal acquisition.Experimental results show that,the traditional LYSO:Ce scintillator has a rise time of(273.7±26.9)ps,while the emerging all-inorganic perovskite scintillator CsPbCl3 exhibits an ultrafast rise time as low as(209.6±6.7)ps and a decay time of only(663.4±34.2)ps.This sub-hundred-picosecond rise time and ultrafast response characteristic highlight the great potential of CsPbCl3 in the field of gigahertz high-repetition-rate ultrafast detectors.It provides critical technical support for bunch-by-bunch diagnostics in synchrotron radiation and free-electron laser facilities,while also offering key methodologies and physical data for the screening and optimization of next-generation ultrafast scintillators.

陈振华;杨帆;陆彦宇;郭智;刘海岗;张祥志;邹鹰;王勇;邰仁忠;丁栋舟

中国科学院上海高等研究院,上海同步辐射光源,上海 201210南开大学物理科学学院,天津 300071中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院上海应用物理研究所,上海 201800||中国科学院大学,北京 101408中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院大学,北京 101408中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院大学,北京 101408中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院大学,北京 101408中国科学院上海高等研究院,上海同步辐射光源,上海 201210中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院大学,北京 101408中国科学院上海高等研究院,上海同步辐射光源,上海 201210||中国科学院大学,北京 101408中国科学院上海硅酸盐研究所,上海 201899

数理科学

钙钛矿闪烁体CsPbCl3上升时间高重频X射线探测器吉赫兹

perovskite scintillatorCsPbCl3rise timehigh-repetition-rateX-ray detectorgigahertz

《人工晶体学报》 2026 (2)

182-190,9

国家重点研发计划(2022YFB3503900)

10.16553/j.cnki.issn1000-985x.2025.0201

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