首页|期刊导航|分析测试学报|融合多尺度注意力与领域对抗学习的铝土矿近红外光谱跨设备建模

融合多尺度注意力与领域对抗学习的铝土矿近红外光谱跨设备建模OA

Cross-device Modeling of Bauxite Near-infrared Spectra via Multi-scale Attention and Domain-adversarial Learning

中文摘要英文摘要

该文提出了一种融合多尺度注意力机制与领域对抗学习的跨设备建模方法.在特征提取阶段,构建结合卷积块注意力模块与多尺度特征融合的一维编码-解码网络,以同时捕获光谱的全局趋势与局部细节特征并抑制噪声;在迁移策略上,引入领域对抗学习,通过梯度反转层与领域分类器的对抗训练实现源设备与目标设备特征分布的端到端对齐,并结合标准正态变量变换与Savitzky-Golay卷积平滑提升光谱输入的一致性与信噪比.在基于两台便携式近红外光谱仪采集的1 330条铝土矿光谱数据上的八折交叉验证中,该方法在目标设备上的决定系数达到0.860 3,均方根误差为1.752 1,显著优于传统校正方法和多种深度学习基线模型.特征分布可视化与消融实验进一步验证了多尺度特征融合、注意力机制及领域对抗策略在特征对齐和性能提升方面的有效性.

Near-infrared(NIR)spectroscopy,owing to its advantages of rapid detection,non-de-structiveness,and reagent-free analysis,holds great potential for mineral composition analysis.However,in multi-device industrial scenarios,discrepancies in light source intensity,detector sen-sitivity,optical configuration,and sampling distance among different spectrometers lead to signifi-cant distribution shifts in spectral data of the same sample across devices.Consequently,the predic-tive performance of quantitative models trained on one device deteriorates markedly when deployed on another.Traditional chemometric calibration transfer methods(e.g.,direct standardization,piece-wise direct standardization,and slope/bias correction)rely on linear mapping assumptions,making them inadequate for complex nonlinear domain shifts.Moreover,they require repeated measure-ments of standard samples,thereby increasing application costs.To address these issues,this paper proposes a cross-device modeling approach that integrates multi-scale attention mechanisms with do-main-adversarial learning.In the feature extraction stage,a one-dimensional encoder-decoder net-work is constructed by combining convolutional block attention modules with multi-scale feature fu-sion,enabling simultaneous capture of global trends and local spectral details while suppressing noise.In terms of transfer strategy,domain-adversarial learning is introduced,where adversarial training with a gradient reversal layer and a domain classifier achieves end-to-end alignment of fea-ture distributions between source and target devices.Additionally,standard normal variate transfor-mation and Savitzky-Golay convolution smoothing are applied to enhance spectral consistency and sig-nal-to-noise ratio at the input level.On a dataset of 1 330 bauxite spectra collected using two porta-ble NIR spectrometers,eight-fold cross-validation experiments demonstrate that the proposed method achieves a coefficient of determination(R²)of 0.860 3 and a root mean square error(RMSE)of 1.752 1 on the target device,significantly outperforming traditional calibration transfer methods and several deep learning baselines.Feature distribution visualization and ablation studies further validate the ef-fectiveness of multi-scale feature fusion,attention mechanisms,and domain-adversarial strategies in feature alignment and performance improvement.

徐志彬;许昊;王刚;左玉昊;雷萌

中国检验认证集团河北有限公司,河北 石家庄 050051||中国矿业大学 信息与控制工程学院,江苏 徐州 221116中国矿业大学 信息与控制工程学院,江苏 徐州 221116中国检验认证集团河北有限公司,河北 石家庄 050051中国检验认证集团河北有限公司,河北 石家庄 050051中国矿业大学 信息与控制工程学院,江苏 徐州 221116

化学化工

近红外光谱迁移学习铝土矿多尺度融合

near-infrared spectroscopytransfer learningbauxitemulti-scale fusion

《分析测试学报》 2026 (3)

563-572,10

中国中检河北公司研发项目(2025ZJHBYF004-1)国家自然科学基金(62473368,62373360)海关总署科研项目(2023HK113)

10.12452/j.fxcsxb.25101502

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