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ZnSeTe全彩量子点研究进展及其发光二极管应用OA

Recent Advances in Full-color ZnSeTe Quantum Dots Toward High-performance Light-emitting Diodes

中文摘要英文摘要

量子点发光二极管(Quantum dot light-emitting diodes,QLED)因其低功耗、高色纯度和广色域优势,已成为新一代自发光显示技术.目前,高效QLED仍主要依赖CdSe或含Pb钙钛矿量子点,其重金属带来的环境风险限制了产业化发展.无镉无铅的环保型量子点材料因此成为推动QLED大规模商业化的核心替代方案.在众多候选体系中,ZnSeTe量子点凭借优异的发光性能和独特能带调节机制,可实现从450 nm蓝光到700 nm红光的宽范围连续发射,是最具潜力的单一体系环保型全彩发光材料.尽管如此,ZnSeTe体系仍面临高Te含量引起的晶格应变、界面缺陷及器件电荷传输失衡等技术挑战.本文系统综述了ZnSeTe量子点的合成及其在QLED应用中的最新进展,重点围绕蓝、绿、红三基色发射的优化策略,分析了组分工程、壳层工程和表面工程的作用机理及最新成果,并展望了其在稳定性、规模化合成与器件效率方面的未来发展方向.

Quantum dot light-emitting diodes(QLEDs)have emerged as a promising next-generation self-emissive display technology,offering advantages such as low power consumption,high color purity,and wide color gamut.Currently,high-performance QLEDs largely rely on toxic CdSe or Pb-containing perovskite quantum dots,whose heavy metal content presents environmental risks that restrict industrialization.Consequently,the development of Cd/Pb-free,eco-friendly quantum dot materials has become the core alternative for driving large-scale QLED com-mercialization.Among various candidates,ZnSeTe quantum dots stand out as the most promising single-system full-color emitter,due to their superior luminescence properties and unique band structure tuning mechanism,which en-ables continuous emission across a broad range from 450 nm blue light to 700 nm red light.Nevertheless,the Zn-SeTe system still faces critical challenges,including lattice strain induced by high Te content,interfacial defects,and carrier transport imbalance in devices.This review systematically summarizes the latest progress in the synthesis of ZnSeTe quantum dots and their applications in QLEDs.Focusing on optimization strategies for achieving blue,green,and red primary colors,we analyze the mechanisms and the latest achievements of composition engineering,shell engineering,and surface engineering.Finally,we discuss the future outlook regarding challenges in stability,scale-up synthesis,and device efficiency.

庞可意;野世阳;梁艺;邹炳锁;曹盛;赵家龙

广西大学物理科学与工程技术学院,广西南宁 530000广西大学物理科学与工程技术学院,广西南宁 530000广西大学物理科学与工程技术学院,广西南宁 530000广西大学物理科学与工程技术学院,广西南宁 530000广西大学物理科学与工程技术学院,广西南宁 530000广西大学物理科学与工程技术学院,广西南宁 530000

数理科学

环保量子点QLEDZnSeTe发光性能

eco-friendly quantum dotsQLEDZnSeTeluminescence performance

《发光学报》 2026 (1)

10-21,12

国家自然科学基金(62475054,62165001)Supported by National Natural Science Foundation of China(62475054,62165001)

10.37188/CJL.20250210

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