WSe2/MoSe2横向异质结中的自旋相关光电流特性OA
Spin dependent photocurrent characteristics in WSe2/MoSe2 lateral heterojunction
采用化学气相沉积法制备WSe2/MoSe2 横向异质结,并利用波长为1064 nm的激光系统研究其圆偏振相关光电流和线偏振相关光电流特性.实验结果表明,圆偏振相关光电流随入射角变化呈现奇对称趋势,这可能与横向异质结的对称性降低至C3v点群有关.对线偏振相关光电流幅值L1 和L2 的入射角依赖性进行分析.L1可能来源于线偏振光致电流效应和表面光电流效应的共同作用;L2 主要来源于线偏振光子拖曳效应.进一步研究发现,WSe2/MoSe2 横向异质结的圆偏振相关光电流受到异质结中电荷转移效应的影响,并与WSe2 和MoSe2 之间的电子弛豫时间差异、导带曲率差异密切相关.
WSe2/MoSe2 lateral heterojunction was fabricated via chemical vapor deposition.Its helicity dependent photocurrent and linear polarization dependent photocurrent characteristics were systemati-cally investigated using a 1 064 nm laser.Experimental results indicate that the helicity dependent photocurrent exhibits an odd-symmetric trend with varying incidence angles,likely due to the reduced symmetry of the lateral heterojunction corresponding to the C3v point group.The dependence of the linear polarization dependent photocurrent amplitude L1 and L2 on the incidence angle is analyzed.L1 may originate from the combined effects of linear photogalvanic effect and surface photogalvanic effect,while L2 is mainly derived from linear photon drag effect.Further investigation reveals that the helicity dependent photocurrent in the WSe2/MoSe2 lateral heterojunction is influenced by charge transfer effects within the heterojunction and is strongly correlated with differences in electron relaxation time and conduction band curvature between WSe2 and MoSe2.
许荣智;周宇超;俞金玲
福州大学先进制造学院,福建 泉州 362251福州大学物理与信息工程学院,福建 福州 350108福州大学先进制造学院,福建 泉州 362251||福州大学物理与信息工程学院,福建 福州 350108
数理科学
WSe2/MoSe2横向异质结化学气相沉积法圆偏振相关光电流线偏振相关光电流
WSe2/MoSe2 lateral heterojunctionchemical vapor depositionhelicity dependent photo-currentlinear polarization dependent photocurrent
《福州大学学报(自然科学版)》 2026 (1)
18-24,7
国家自然科学基金资助项目(62074036)福建省科技厅对外合作资助项目(2023I0005)
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